The project Chiral light-matter interaction for quantum photonic devices (AA2-14*, 01/2021-12/2021) is a project within Application Area 2 (Materials, Light, Devices) of the Berlin Mathematics Research Center MATH+ (DFG excellence cluster EXC-2046/1, project ID: 390685689), headed jointly by researchers from ZIB and from TU Berlin (Stephan Reitzenstein).

The objective of the project is to investigate and apply numerical methods for the simulation of chiral light-matter interaction in nanostructures. The main goal is the development of contour integration based methods and their application to topical devices for photonic quantum technology.

We plan to investigate the coupling of quantum dot single photon sources and other sources to experimentally realizable chiral nanoresonators. However, resonant photonic nanostructures typically support a large number of eigenmodes with complex properties, including electromagnetic (e-m) chirality density, quality-factor and mode volume. The interaction of light sources with such multimodal resonators needs to be accurately quantified for interpreting experimental results and for design purposes. For achieving near unity coupling efficiency, the various experimentally accessible parameters of the experimental setups need to be optimized.

Figure 1: Top: A 40nm gold sphere induces plasmonic coupling between two 50nm long gold rods that are arranged in a chiral fashion. Bottom: Corresponding simulated plasmonic field distribution [Top SEM image: T. Liedl, bottom image: ZIB].

Research results of this project include the investigation of long- and short-ranged chiral, electromagnetic interactions in plasmonic nano-assemblies [K. Martens, et al., 2021]. A typical, resonant near field distribution in such a setup is shown in Figure 1.

Publications

2022
Chiral Generation of Hot Carriers for Polarization-Sensitive Plasmonic Photocatalysis with Hybrid Nanostructures J. Am. Chem. Soc., Vol.144, p. 1663, 2022 Yoel Negrin-Montecelo, Artur Movsesyan, Jie Gao, Sven Burger, Zhiming Wang, Sylvain Nlate, Emilie Pouget, Reiko Oda, Miguel Comesana-Hermo, Alexander O. Govorov, Miguel Correa-Duarte BibTeX
DOI
MATH+ AA2-14
Numerical optimization of single-mode fiber- coupled single-photon sources based on semiconductor quantum dots Opt. Express, Vol.30, p. 15913, 2022 Lucas Bremer, Carlos Jimenez, Simon Thiele, Ksenia Weber, Tobias Huber, Sven Rodt, Alois Herkommer, Sven Burger, Sven Höfling, Harald Giessen, Stephan Reitzenstein BibTeX
DOI
arXiv
MATH+ AA2-14
Resonant Plasmonic–Biomolecular Chiral Interactions in the Far-Ultraviolet: Enantiomeric Discrimination of sub-10 nm Amino Acid Films Nano Lett., Vol.22, p. 7343, 2022 Tiago Ramos Leite, Lin Zschiedrich, Orhan Kizilkaya, Kevin M. McPeak BibTeX
DOI
MATH+ AA2-14
Toward maximally electromagnetically chiral scatterers at optical frequencies ACS Photonics, Vol.9, p. 1954, 2022 Xavier Garcia Santiago, Martin Hammerschmidt, Johannes Sachs, Sven Burger, Hyunah Kwon, Marvin Knöller, Tilo Arens, Peer Fischer, Ivan Fernandez-Corbaton, Carsten Rockstuhl BibTeX
DOI
arXiv
MATH+ AA2-14
Visible wavelength spectral tuning of absorption and circular dichroism of DNA-assembled Au/Ag core-shell nanorod assemblies Mater. Adv., Vol.3, p. 3438, 2022 Mihir Dass, Lilli Kuen, Gregor Posnjak, Sven Burger, Tim Liedl BibTeX
DOI
MATH+ AA2-14
2021
Deterministically fabricated quantum dot – waveguide systems for on-chip quantum optics Proc. SPIE, p. 118060G, Vol.11806, 2021 Peter Schnauber, Johannes Schall, Samir Bounouar, Kartik Srinivasan, Marcelo Davanco, Jin-Dong Song, Sven Burger, Sven Rodt, Stephan Reitzenstein BibTeX
DOI
MATH+ AA2-14
Long- and Short-Ranged Chiral Interactions in DNA Assembled Plasmonic Chains Nat. Commun., Vol.12, p. 2025, 2021 Kevin Martens, Felix Binkowski, Linh Nguyen, Li Hu, Alexander O. Govorov, Sven Burger, Tim Liedl BibTeX
arXiv
DOI
MATH+ AA2-14